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Native CuA redox sites are largely resilient to pH variations within a physiological range

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Chem. Commun., 2013, 49,5381-5383
DOI: 10.1039/C3CC40457A, Communication
Damian Alvarez-Paggi, Luciano A. Abriata, Daniel H. Murgida, Alejandro J. Vila
The redox, structural and spectroscopic properties of native CuA sites are not affected by pH changes at a physiologically relevant range, contrary to what has been observed on engineered CuA sites. This challenges the notion of a previously proposed pH-based mechanism for the regulation of electron transfer reactions of cytochrome c oxidase in vivo.
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