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A novel nonanuclear hafnium oxide-hydroxide-sulphate cluster crystallised from aqueous solution

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Chem. Commun., 2014, 50,997-999
DOI: 10.1039/C3CC48167K, Communication
A. Kalaji, L. Soderholm
Single crystals of (NH4)14[Hf9O8(OH)6(SO4)14][middle dot]nH2O (1) were obtained by heating a sealed aqueous solution of HfOCl2[middle dot]8H2O, (NH4)2SO4 and H2SO4 at 80 [degree]C for 10 days. The discrete [Hf9O8(OH)6(SO4)14]14- anionic clusters have no inter-cluster connectivity. This rare nonameric architecture has only been observed previously in two Bi3+ oxo clusters.
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