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Evidence for the formation of a metal alkyl intermediate in the zinc mediated intramolecular hydroamination

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Chem. Commun., 2013, Advance Article
DOI: 10.1039/C3CC45491F, Communication
Sankaranarayana Pillai Sarish, Dirk Schaffner, Yu Sun, Werner R. Thiel
The zinc catalyzed hydroamination of 2,2-diphenylpent-4-en-1-amine stops at the alkyl intermediate! A bulky [small beta]-diketiminato ligand prevents transfer of NH protons to a carbanion, and the formation of a long-time postulated intermediate of catalytic hydroamination is proved.
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